Table of Contents
This section depicts the structure and relatedness of fuel cell R&D,
with particular emphasis on the question: "What does fuel cell technology
research look like?"
Technology Mapping Analysis
Principle components analysis was conducted on 200 leading keyword terms.
Fig. 14: Fuel Cell Technology Map
Technology Clusters:
Five types of fuel cells, distinguished by type of electrolyte material
used, dominate current research and development activities.
Phosphoric Acid Fuel Cells (PAFC):
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Status: Pre-commercial/commercial; The most mature commercially available
fuel cell technology (under development for over 20 years with total worldwide
investment in excess of $500 million). Largest unit installed: 11,000kW
(200kW units in commerical production).
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Phosphoric acid is used as the electrolyte and natural gas is used as the
fuel.
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They operate at about 400 degrees F, and their electrical efficiency can
exceed 40% LHV.
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Reforming of the natural gas feedstock to a hydrogen-rich gas occurs outside
the fuel cell stacks.
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Due to PAFC complexity, projected capital costs are high ($1,200-$1,500
per kW) and efficiencies are low.
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Currently being used in many different types of buildings, ranging from
hospitals, hotels, power plants, and an airplane terminal. Possible future
applications include buses and locomotives but probably not smaller vehicles.
Molten Carbonate Fuel Cells (MCFC):
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Status: Pre-commercial; Now being tested in full-scale demonstration plants
(e.g., Santa Clara Demonstration Project). Largest unit installed: 2,000kW
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They offer higher fuel-to-electricity efficiencies (approaching 60% LHV),
and operate at higher temperatures (1,200 degrees F).
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Utilize a lithium/potassium carbonate electrolyte and nickel electrodes.
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Reforming can occur inside the fuel cell stacks.
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Main problem with operation and manufacture of MCFC's relates to the design
of electrodes; must withstand working for long periods in the electrolyte
which is hot and corrosive.
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Projected capital cost: $1,000-1,200 per kW
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Seen as an ideal source of large scale power generation.
Solid Oxide Fuel Cells (SOFC):
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Status: Developmental; Currently being tested in a 100-kilowatt plant.
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They offer the stability and reliability of all-solid state ceramic construction.
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The electrochemical conversion process occurs at very high temperature
(up to 1800 degress F) and so supports internal reforming; allows more
flexibility in the choice of fuels.
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Moderately high efficiencies (approach 60% LHV) with a high-grade waste
heat product; potentially the most efficient type with very useful waste
heat.
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Three fundamental designs - tubular, planar and monolithic types
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The materials used to make the cells are very difficult to produce, and
their manufacture at reasonable cost is a problem yet to be resolved.
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Projected capital cost: $800-$900 per kW
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Suited for applications requiring a large amount of power including industrial
and large-scale central electricity generating stations.
Proton Exchange Membrane Fuel Cells (PEMFC) or Solid Polymer Fuel Cells
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Status: Pre-commercial; PEMFC buses operational by Ballard Power Systems
in Vancouver.
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Use a polymer solid-state electrolyte and platinum electrodes. Membrane
is made of polyperfluorosulfonic acid (similar to teflon). Pure hydrogen
is usually used as the fuel but natural gas and methanol could also be
used.
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Low temperature cell operating at about 200 degrees F.
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Principal issues related to costs are focused on the electrolyte, known
as the 'proton exchange membrane' (PEM) and the bipolar plates.
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Showing great potential for light-duty vehicles (cars, buses), buildings
(heater/chiller units), and very small scale localized power generation
(replacement for rechargeable batteries).
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Direct methanol fuel cells (DMFC) are PEMFC's which use methanol directly
as a fuel.
Alkaline Fuel Cells (AFC)
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Status: Pre-commercial/Commercial; used by NASA for many years
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Potassium hydroxide is used as the electrolyte and hydrogen as the fuel.
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High power density and high efficiency (up to 70% efficient).
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Production costs high due to precious metals required on the electrodes
(platinum, palladium, gold).
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Problems with corrosion, contamination, and carbon dioxide waste products.
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Very small niche market of power supplies for space vehicles.
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Possible uses in land vehicles and submarines
Application Clusters:
Materials
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The use of different materials in the electrolyte is the major distinguishing
characteristic of fuel cell types.
Spacecraft
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Primarily powering space shuttle and related machinery.
Transportation
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Fuel cells can be applied to four different transportation segments--buses,
fleet vehicles (including trucks), passenger vehicles and locomotives.
Cogeneration Plants
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Fuel cell power plants principally for electric power generation
Mathematical Models
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Techniques to improve fuel cell efficiency and performance.
Marketing/Economics
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Issues in cost, feasibility, and viability in commericializing fuel cells.
Environmental Protection
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Emphasis on reducing emissions by replacing fossil fuel consumption.
Technology Decomposition
Co-occurrences and cluster analysis can be conducted on specific technology to
decompose the supporting technologies, materials, processes, and applications.
The results of the decomposition of solid oxide fuel cells is shown in Fig.
15.
Fig. 15: Technology Decomposition - Solid
Oxide Fuel Cells
The prominent keyword terms match the general literature on SOFC's.
The solid oxide fuel cell uses a ceramic electrode of yttria-stabilized
zirconia operating at about 1,800 degrees F. The oxide ions, transported
through the electrolyte combine with hydrogen at the anode and produce
water vapor and release electrons to the external circuit. While in the
cathode, oxygen combines with free electrons to produce oxide ions. Carbon
monoxide can also be used instead of hydrogen in these fuels cells to produce
carbon dioxide and electrons in the anode.
Of primary importance, is that the electrolyte is in a solid phase and
not a liquid electrolyte with its attendant material corrosion and electrolyte
management problems. The solid state character of all SOFC components means
that, in principle, there is no restriction on the cell configuration.
Instead, it is possible to shape the cell according to criteria such as
overcoming design or application issues.